: s srngdeonn ti i atda tx gnnwlaenie Ae ailILmrt cp ioeemdPMpoeSCS-lateM noita inc m ee rupg de lSnn to aAaCrhWe ctxaEW/tn es mn rioo diFetSacilpmI nhoJ .Rt anoD egidruB .dJivaD yrtsimehco idB nyartsim e f h.oCtpeD cirehps o,dmhn tta, Arn.a atEfepoceOD secneicS y tisrevin Unoinimo DdlO ytisrevin Unoinimo DdlO ,k2l1o 0fA-rV9o2N532 6 ,6k7l2o 0fA-rV9o2N532 Phone: (757)683-409 8 Phone: (757)683-4930 8 2 6:4X-A3F86)757( 30 3:5X-A3F86)757( ude.udo@TANO: DlJiam-E ude.udo@EGID R:UlBiDam-E t n9ra9er8bG0m-u1N-3 9-41000N mth.jhagprno/naeco/hcet_ics/lim.yvan.rno.www//:ptth LONG-TERM GOALS e hnytia lnpoitaice pd snnaoitaxelpm otca hetl oe rhetnimret eoe dtrsala omgret-gn orluO -lat e fmeocnatrop mei hdt n,asnoitac ollatsa odc neaniraut s nesilat e fmeognahc xreetaw/tnemides ,lac o nlnooitaice plsat enmmul orcet a owstretawer oepniraut smeo rgfnixu lsfdnag iglnixelpmoc .sela clsabo ldg n,alanoiger SEVITCEJBO detcel efnsooitaice pe shd tnnaoitaxelpm oftconet xe eh:) te1n(imret eoed trsaevitcej bcoifitnei crsuO -l a stfheotmgne rdstnnsaoitart n;esc rn)eo2tc(awe rtonpemi ddsenrsae tmao wt stnloia bteecmart e hfntooitcer id dneaduting ae mh) t3;(sretawer otpnemid ed snsaret amwott onsbidnag iglnixelpmoc sretawer o fpto ugonixu lsfdnag iel h fteocnetsisr eep h)t 4 d(; nsadnag irlie hdt nsalat e fmxou lcfihtneb .sessec olrapvo m dennroaitadar greid e dhsntrae tmaowt tgonbiylr eovtoni HCAORPPA hcrae sr eudroeft c.us d t, ner8 nowo9 YIcf9yFf1reotaro bddanl l aeh sitftfoosbis nhoccaor prpuaO eniraut so ewmto rnfmul orcet ad wnsaretawer otpnemid ee shdtelpm ae,sw7 9r‘ebm e.v soneNIsiurc ,hc r. as nMcIitsiretcara hlcacisy hdp nlaacimehcoego igbnitsartn ogcniv a,hy aeBkaepase h nCsietis ar(ev ihRtebazi leE hmto rnfmul orcet adw nsaretawer otpnemid ees hdtelpm a es,w8 9y‘l udJ n,alirpA nsoeidu tysrotarob arl udoeuni t. n) o recoWbr alhav a SNrUoj a,mdetcapmi-yllacinegoporht nyalhgih slfeao ltioft orreptawe rdoepnimre t.eenWdoitadar g deendcanetsis rdenpa gduieClvired-retawerop n fZsotnatsn oyctiliba tlsanoitidn oec hdt nsanoitartnecn odcnag iglnixelpmoc- ndZ n nadZevlossid nd Z nudaCevloss ild a fts ooetlifo rrpetawer odpenimret ee.dWset iy saeBkaepase he C htstaexelpmoc ndZ n ua fCsotnatsn oyctiliba tlsanoitidn oec hdt nsanoitartnecn odcnag iglnixelpmoc- ndZ n uadCna .et irsev ihRtebazi leE h ttsaexelpmoc -di cgani sduelpmasb uds n,arer oxc osbsalgixe l rploee tssselnia tgasni sduetcell oecr eswtnemideS rNed nduenoitc eesr eswer otcnem i.d seeSb uetr oscsalgixe ldpenaelc er eswlavret ntinemid eds na 2 la t rosoteflpmas b;u)smµ54 .d0e(ret lei rfseewlp mraesta w.es reorPutarep mue ttdtnieaisgufirtnec Report Documentation Page Form Approved OMB No. 0704-0188 Public reporting burden for the collection of information is estimated to average 1 hour per response, including the time for reviewing instructions, searching existing data sources, gathering and maintaining the data needed, and completing and reviewing the collection of information. Send comments regarding this burden estimate or any other aspect of this collection of information, including suggestions for reducing this burden, to Washington Headquarters Services, Directorate for Information Operations and Reports, 1215 Jefferson Davis Highway, Suite 1204, Arlington VA 22202-4302. Respondents should be aware that notwithstanding any other provision of law, no person shall be subject to a penalty for failing to comply with a collection of information if it does not display a currently valid OMB control number. 1. REPORT DATE 3. DATES COVERED 1998 2. REPORT TYPE 00-00-1998 to 00-00-1998 4. TITLE AND SUBTITLE 5a. CONTRACT NUMBER Metal-Complexing Ligands And Metal Speciation In Sediment 5b. GRANT NUMBER Porewaters: Implications For Sediment/Water Exchange And Water Column Speciation 5c. PROGRAM ELEMENT NUMBER 6. AUTHOR(S) 5d. PROJECT NUMBER 5e. TASK NUMBER 5f. WORK UNIT NUMBER 7. PERFORMING ORGANIZATION NAME(S) AND ADDRESS(ES) 8. PERFORMING ORGANIZATION Old Dominion University,Dept. of Chemistry and REPORT NUMBER Biochemistry,Norfolk,VA,23529-0126 9. SPONSORING/MONITORING AGENCY NAME(S) AND ADDRESS(ES) 10. SPONSOR/MONITOR’S ACRONYM(S) 11. SPONSOR/MONITOR’S REPORT NUMBER(S) 12. DISTRIBUTION/AVAILABILITY STATEMENT Approved for public release; distribution unlimited 13. SUPPLEMENTARY NOTES See also ADM002252. 14. ABSTRACT 15. SUBJECT TERMS 16. SECURITY CLASSIFICATION OF: 17. LIMITATION OF 18. NUMBER 19a. NAME OF ABSTRACT OF PAGES RESPONSIBLE PERSON a. REPORT b. ABSTRACT c. THIS PAGE Same as 6 unclassified unclassified unclassified Report (SAR) Standard Form 298 (Rev. 8-98) Prescribed by ANSI Std Z39-18 er eswesyla nnaoitaice pds nnaoitaxelpm olcat erm osfelpmasb u;s )H2 pd(eifidi cear eswlat edmevlossid citlatsir ehapt idwetcell oecr eswelpm ansmul orce t. asWisyla nlait nkur add ndal o,ccixo ntapek en i nldieretl i,f”enav-hsi fc“itsa ldpethgi e oawdtehcat tganib untolf ehTguor hmtets ygsnipmup . H 2opdteifidi cda n,anoitcell ogcnir u)dretl imfµ22.0( tnemid edsetcell oyclhse rgfnid d yadbetagitsev nsi aswdnag i uldCevired-retawer o fpeocnetsisr eephT e.sr ee htmTaowt teo tbginsilp m ehashtsatgne rctis neo m ienafhosotitu lsloo rCtsaeatNawerop ndaoenoitis o,pseltt onbolf eL T-d2enaelc-di cndaietabuc neir eswlortn odcetaicos sraie hd tnsaelpmas yaybad/sru o 2hr1 odfetaidar reir etwhg i oldtesop xseelpm ae.s hhTcn erbia-nae lnaecolb artekahs kca l fbsorey allarev ehst itwhg imlo rdfedlei hesr eswelpm aks r. apDm anlegolah/netsgn utttaw-57 yad- 9 o 3 0tra3e vsoeuqinhc entae llcat eemca rgtni sduelpmasb uesr eswnoitul o ls. lsAg acbitsalp .ytinil ads n,a H,p O,DC O,D udCevloss ildat o,tsdnag iglnixelpmoc- urC odfoirep retawer odpetcell oyclhse rgfnid dydabemrofr eepr esweidu tnsoitadargedoto hdpnag iglnixelpmoc-uC ne hetr eswelpm aess e. hrTet amwott oebt igsnilpm aes h styatinil aesm aes h ftsonoitul olsC aoNt - rudoCeflpmas- beu rssenwoitu l eo.sss erh uT rpo2opout2h mfcarla -dy 2Wgeba.kHt1aidarri ,H H,pC O,D udCevloss ildat o,tsdnag iglnixelpmoc O .ecnabrosba-siV/ Vd Una 2 2, d naadnu Se(cnecsenimulime h ycdbenimret eedr eswnoitartnecn o)cuCD T u(dCevloss ildatoT esl ulpaitnereff i yddbenimret eedr eswnoitartnecn o)cnZD T n(dZevloss ildat o;t)19 9,1namstnuH - nd Zn- au.C)pe rntpipircsun ad mn7a9 9,1yrn ed Hntaan o;DVSAP Dy(rtemmatl ogvnippir tcsidona gnign a tahVaSA P yDdbenimret eedr eswtnatsn oyctiliba tlsanoitidn odc nsanoitartnecn odcnagil esfhtotnats nyotcilib altasnoitid n dosncnaoitartnec n;o)c4 9, 9 .t1tlaean oeDd(ortc epl oeyrrducrem gnippir tcsidoht aecvitprosda/noititepm odcnag i yldbenimret eedr edwnag iglnixelpmoc- utCsegnorts h dgyeibnhimre te ersdenwoitartnec nCroOecDt a.w)e 4r 9o , 9Pt.t1alena oyDr(temmatlov ,stneir t,uendif l ,,urneseMFtawe r;o)p4 9,9d1aets mdeongHaidr unBo(itad icxiotyla tearcutarepmet dn3a OC . sdoht edmradna tydsbenimret eedr ew 2 KROW DETELPMOC dnag iglnixelpmoc- u,Csnoitartnecn oucC DdTenimret eedv a eh,wstrof f’esra elyacs isfuoive rep hntI y aeBkaepase hfsCoretawer otpnemid ee shnntioitaice pd snnaoitaxelpm oud cCn,asnoitartnecnoc udC nuaC D fTxou lcfihtn eeb hdtenimret eedv a ehdw n,a7 CeWt ifSle hlsatnenitn odc n ,a ,SsMetiS dnag i nl,Zsnoitartnecn oncZ DdTenimret eedv a. edhS WnsMaet ieSkaepase hmCo rsfdnagil . ey WaeBkaepase h fCnomul orcet aew h ntnioitaice pds nnaoitaxelpm o ncdZ n,asnoitartnecnoc eyh d ttuonttesmire pedxneeote l.p r m oa rosseeecnlyWpoas a3se-es2id uets sedhettcudnoc .nmul orcet aew h ntsidnag iglnixelpmoc- udCevired-retawer o fpeocnetsisrep -dueCvired-retaw e erfcoonpetsis rnempuloc-r e ytefd ahoud wttndso ecatee sl np ,YIme8Fow9c .sdnagil- ufnCooitadargedoto he phott nnioitagitsev nneiadulc noyitdu tssi hdtednap xede wn,asdnagil gn ow loehtamit sspeul eodhtengis eedr eswtnemirep xneoitadargedoto hd pneacnetsisr edpnag ielsehT odt n,anmul orcet aew h nttisisr etphg ismretawer otpnemid emso rgfnixu lsfdnag iglnixelpmoc-uC . nmul orcet aew h nt ui fCnooitaice pds nnaoitaxelpm oec hetcneulf ntihg iyme httnet xteahw ,,nlZa teec matrntatro prmeiht od,nnraae vhitRebaz ie,lheE tttinsatro prmeiht odn e an,dYeI8dFw9a dd-,fnnunoa aCZ,D u TsCfeDoxT urleftawe rdoepru s ,aerewem vhitRe b.asz e ieinlhdIE t urotutso dnagil- ndZ nnaZ D fTsoelifo rhptp erdetawer odpenimret eods l. easWdnag iglnixelpm oncZ set iy saeBkaepase hhCt otsbaexelpm o nfcsZotnatsn oyctiliba tlsanoitidn oe chd tn,asnoitartnecnoc .et irsev ihRtebazi leE h ttdana e,wsdnag iglnixelpmoc-lat efnmooitcudo re phnstiesseco rtpnemid efesol oe rhdtnatsred nruett eobT e w,yllacifice p .Sstnemide senira mn ignilcy cretta mcinagr odevlossi dydut so tdeunitno cosl aevah noitanoitca refz iCs O nDdoesa bs(tnemid eesnir a nmginilc yMc OrD olfed olmautpecn odacepoleved devloss ifsdoeidu tdsemrofr eepv a,hyltnec etrs o,md n)a89 9,1rendr ad Gneagidr u;Batad er otpnemid eesnir anemicnecserou lM fOd Dn)a89 9,1egidr ud Bnraendra Gs(etardyhobrac .) 8,9e9g 1i n ddesrnhruaCeB(taw stpircsun agmnirape re prrdaoettimb uesv ad hn,asgnite elmanoit atsnatlus er rudoetnese repv aehW fle hlsatnenitn odc neaniraut s nesidnag iglnixelpmoc- udC n ua fCyortsimehcoego ieb h)t 1:(no mo rsfdnag i ul fCxou lef h)t 2;()weiv e nrtipircsun a,megidr udB n,atan o,Dlabark Ss(tnemides ,-dueCvired-reta we ecfrnooeptsi s;)er)3he 7(tp,9e9g1i d,drtnu aaB,nloaDba rsktSn(em iedneisrautse ) 4;().pe r nptipircsun adm n;a89 9,1egidr udB ntaan o,Decir Pn(mul orcet aew h ntsidnag iglnixelpmoc d n7a9 9,1yrn edH ntaano Dn(mul orcet ayw aeBkaepase heC h ntnioitaice pds nnaoitaxelpm oncZ rev ihRtebazi ldE nya aeBkaepase h nCnioitaice pds nnaoitaxelpm o nc)Z 5;().pe r nptipircsunam mo rsfdnag infxlZou le fh) t6;().pe rntpipircsun ad mn;a89 9,1egidr ud Bntaan o,Dsrey Bs(retawerop devloss i) d7;().pe rntpipircsun ad mn8a9 9,1egidr ud Bn,atan o,Dsrey Bs(tnemid eesnirautse ) d8;n()a.p etnrpipircsu n da8nm 9a,9e1gid r durnBeandr asGr(etawe rtonpemi dsneeistardyhobrac .).pe rntpipircsun ad mn8a9 9,1egidr ud Bnnaeh Cs(retawer otpnemid enesicnecseroulf-MOD STLUSER -ecnetsisr edPnag iuLC s-feuosCs aele crth s tdateeanliat nsorce tma owet ttyMeioakSbBaepas ehC ,Lssa ldcnag itlsegnor tes h ftnooitartnecn oe.c hsTdnag iglnixelpmoc %1 1d-e3si r g p’ o mK)l~o5(c1 1 sLessa ldcnag irleka ee whstaere h,wlo odpnag iullCat oe thfto d n)a2 L1’g~Ko l( )g’8oK~l( 2 3 udCevloss ildat of%to9. 9n9a hr te.t lao e odrpnGag iue lChf%to79- 9g8niniam ee rhdtesirpmoc ydLbexelpm os cauwC Df%To8 8d ~n,adexelpm oycllacinag rs oaswret amwott oe b hn)tiuCDT( . 1 L ,noitabu cynaid - e0gh3nti rtundats nyolcevita lee rrselwort nroec tmaowt tsnoniboitartnec noc 1 r emtLoa tw ttgaonhbittacidni .Lsela cesm ietlbaicerp pneaodarg et dosne od snoitartn ecnoc 1 1 -retawe rt oagphntitseg g, uk dsreneahitdtabu csnrie tmaowt tdoebkips-retaw e yrnloitphg idlessaerced dLevired ,rLeve w.o)H s nyn0oai3idtcu d7M e.nkr4 r (etanhndite te x meeoodtsar g yeadm 1 1 n.Ithg indlietabuc nsiret amwott odbekips-retawer onypilbaicerp peasaerc et dod nisdnoitartnecnoc ,tcaf eht gnortsL ydbesaerc nyillaut cnaoitartnecn orcie h,tnoitabuc nginir uddetsisr eypl nto osndnag il 1 -retawe rdnoeipvre s sbtaolwu srearl i. mnAiositcud olrapcigol o eoiyutbldbab o,r oprfwoot tr ceaavfo dLevired-retawer otpa hettacid nsitlus eer s.e thhTg indlietabuc nsinoitul olsC adNekips eh ts(dnag il 1 ,re tganwiylr eeo vhtdotneitropsn ae rc, tndtonnaetsis re)erspas adlnca gtinlatro pt msdtionsmaegnorts .selacsemi telbaicerpp an oniamer eng i neL raloohtn ctdielw orhestawe rdo e pddfidooa vseedlp mrae stmaowttoB noit arretvnoecnoc 2 mot tdoebkips-retawe rdnoeipvre s sbdaonw eerctnetsis ree mp ea.hsdToi rneopitabu c yne0aih3dt , y0r a2ed t.LfnAoitab u sc ype0ornfauh2teiodttaw no ifto a.dLe a strda hge egerorid atcleeSpdpa 2 2 dLevired-retawer ofypotiroj ae mh.Tsnoitul olsC adNekips-retawer ondpietacid nois lsaaw sdnagi l 2 .)ylevitceps e ,8 rd% 97n %8as(noitidn okcr ad dntahg ihlt orbed nsuy a9rd3et fdaeniamer ,Lssa ldcnag itlseka eewhT sneimi gke rr datndha ghi tlroeb dsnluort nroec tmaowt tdnoeibtsis r,ep 3 r Lodfeniat bsotlus ehrt itwnemeerga dL na . emoLS 0 t2%n0h(i3 ghi tldnoeibrru cncooitadar ged 1 2 3 laiLtnat s eb.rusosrM emtoa twdteokbips-r e kt)2dras1n awy(a% d ea)nrd sio0yp3ad noita darged 3 ;4 s5%fnoLoitu llo CsdaeNkips-retawe rdnoeipvre ssbaow dedar g 6d e%7ntdahg ie lhndtiedarg ed 3 n i e khrrte a v.d9os3ya d str aatheItpLpa soustC adlnca gtinlatro ptmsi a detnlsaek a ee,hwt 3 .selacsem ietlbaicerp pnsaotsis r 5 e%3t p~u,bsedarg e,dnoitaiceps - r0eo3rfeves rsedpna gduieClvired-retawe rto apdhettartsno msetdnemire pexcenetsis rdenpa geihlT ret ayw aeBkaepase h sC.Aret amwott ogbniylre veo hott nxiu ldfetalum irsie hgtniwoll osfy a9d3 noitad a,r )ga4e 9dt9a1n oe Dmr( iegtvnoisae rr ocaetneb i pstopnodaonitartnec ndonc a ngumiCulloc gn ifdoenhatt s r r.eres hudnotonoTruiutfartn e ecytn daoeatc ves trtyts esasioswuxtehmertpap ts oem hdteidu t ens,wmul orcet agwniylre veo h otstdnag i u lfCsoexu lrfetawer o fpeocnacifingis .noitadargedot o,hypawh tnaopitadar gyeldekil noitadarged odt nouahCgPiL sdnagi ld-euvCired-ret anw oefirotoaprtne c-l ,naedothe cotttc espAxe L( noitadargedo tro ehtd psrlroaitfn e .meeihcrT re tupd hoxecogsesrti oa lnap-dexgeheHswae r)ced T de toa t le eut sbca9alr.wa1 cx01 -4 s-1 . We corrected this rate constant for: (a) the strength of the Hg- -yllacimehcoto h,pdegareva-yllabo l)g b,()yrtemonit cganis ut(hgiln unso o ondterapm opcm aclra tnats ne otdcaert c.enr mreu ohlrcT oe tct enh anhigfwotioiltaune te)d,thcneat(acnaida rtrniaveler 6.8( x01 -8 s-1 ekaepase heC h ntsidnag idlevired-retawer oep hrt osfy a5d 3 f1eom ietcnedis edaredle i)y ekaepas ernhei C tefa moweictnedi s eeehrct n.inSoitadargedot otohctpep she tr,inwmu lroec tyaawB udCevired-retawer oe phfetom ietcnedis ee rh,t).mm o.csr e,pnosniveL-ella Vs(htn o2m1 -sy9iaB deuvCired-retaw ene rosfoi eopthh cgte augaror fhatstlatlhsate g,gnuositadargedo tr oe,htspfdanagil ecru ossi hmto rsfdnag iel h fttorop xtenacifing i,asyraut see hntiht idwedargedoto h epyb asmdnagil .ru cye canlomoazts aeoohtctni sdnagiL- ndZ n nadZevloss ilDatoT ndietcell oscretawer oy paeBkaepase hnsCinoitartnecn oncZ D-T e hfm tocr2ep pe uhnstinoitartnecn oncZ D,Ty a d B.ie Mmhn n t Im0-~o 65rdfegn a7r9 9r1ebmevoN sre t)aMwne0r1o~p (erew x01 ~retaer gnaht ni mot t,osbretaw dn adeniamer ta 5~ ot Mn51 nwodot m ohy r m t tas encenteuB nnerpa2hiohos oihephtbtsa2i ttutw~to aatxer3rtgne c nn.ZomDccT51 deg nsarretawe rroe pvhitReba z sinnlioEitartnec nn oZ. cDm M Tctn d5a0oe12ts~aer cd,ensdaretaw sretawer orpev ihRtebazi leE h ntniZ D.Ty aeBkaepase heC h otrtalim isselifo rhpt i,wMn0 5-3 1m~orf .m cr2ep peu h nttisehg ishaw sretawer orpev ihRtebazi ldE nya aeBkaepase heC h ftsolavret nriep peu h ntsinoitartnecn odcnagil-nZ 0 1fs~otnatsn oyctiliba tlsanoitidn ohct i,wMn00 0o02t0 7m~o rdfegnar 7 dnagil -rneZtawe r.oP .snoi t a sreesthg e nTrrc fmre aexnoonecxlteatZtn0ahtDao 0etoTwcs 0rbne1gor-ie0tw0a1rtnecnoc d n ne Z f acyDsoeraT rbumaeotsawe rt oatphsteg gsursetawe rsenonhipotitartnec ndoncagil -dnnZa rev ihRtebazi leE h ntsiexu ltfnemid edsnagil- ndZ nna Z. DsTret amwott ogbniylre veo h otstdnagil-nZ yltnerr uec r8a9 9e1n u nJdietcell oscelpm ads n,a89 9l1ir p nAdietcell oscelpm agsni sduezyla nearew 899 1lirp Aeh tmor fata dyranimile r .Psdnagil-n Zdn anZD Tf osexul fetagitsevn io tdezylan agnieb o,tsdnagil- ugCnor tysr ed vn,asdnagil- nhZt ofebocr u doaesed ne irsatnemid ee shtta hwto hssexulf .nZ DrT okfn i sasta cya armev ihRtebazi leE h ntsitnemid ees htta hdt n,aret agwniylre veoht Porewater DOM dte ui nors d ire tr eYai rdsesw FcdMeneh uoe8uOtattolv9tDartlasw uahe-froP e e os;s 8l9a 9,1rendr ad Gneagidru Be(vo bdaessucs ilded oymtivitca eerz irsetawer oe phetnimaxe ralucel owm oel htta hdtevres beov a eh,wyllacific e. p)S89 9,1egidr udB n8a9 9,1gne hdZ neagidruB ekil-"cimu hs"tibih xyeltnanimode rhptp ehdt igwnitalumuc cMa OrDetawer o)pa D <3kt(hgiew ndiemusn od cndaecudo rhpt osebicnecserou lefkil-"nietor ph"t iM wOtDa hd tn,aecnecseroulf r ao etreMpebOptDaa wt enfreoo tpentoacrdyho blr aatdtchno gatria el.wusct enelehomTmides d nsaetardyhobr aeclbazingocer-yllacime htca httsegg ussnoitavres beose hrtehteg o.Tdetal eyrlesrevni ese htta hdt n,aM O fDnooitca rtfhgi erwalucel ohmg ieh h ntdinu oyfllaitnerefe rep rsaeditpep/snietorp w oylrotcarf eonrtw ondeko rrbehtr ursfotneirt ucninagro noditezilarenim eerrbeht iy easmlairetam .srosruce rlpacimehco irbie h stealbazingoc eyrllacime hrcegn o ol sntia hMt OtDhgi erwalucelom TCAPMI d ntanet xe ehgtnillortn oy cbe(t arfie hhtt osbnrev osgretawer otpnemid enssilat efnmooitaice peshT y ba(to i nbsotcef freie hdt n,a)nmul orcet aew hdt nsatnemid enseewt egbnilc yrcie h ftdoeeps hg iyhr enviatn oscretawer otpa hettacid nsitlus e rr. u)Oyticix odt nnaoitalumuccao igbnicneulfni hci h,wsdnag inglZnorts-yletared od mnsadnag iuglCnor tysr ef)voralomorc iopm tus(noitartnecnoc ugCnor tysr ee.v hsTlat eom wetse h fteognahc xreetaw/tnemid ees hetcneulf nyildekr admluohs ts or mu.Onmul orcet agwniylre ve ohott nsiretawer oe p hftt ou xo,u sldfnag inel Zhd tn,asdnagil s($doir eepm ittnacifing ir sosfret amwott ontbisisr espdnagil- ue Chtta hettacid nsitlus etrnecer 30 noitaxelpm o ucgCnicneulf nyillaitnet ospu h,tyraut see hetpac s oehtguo ngen otlsisr ehpci h,w)syad .sre t)anwa enc eosppoah rde nplaa(ts annooicitaic edpnsa STCEJ ODREPTALER stnemid e nsginilc ylcat edm nsaisenega icdinag r nosotcejo rRp NrOeh ttonemilpm osctlus erruO nmul orcet aew h ntsilat eemvitcao i fbnooitaice plsacimehc-ocisy h,p)ela odC nnaosnh o,JnoslereB( evit ce.av )aeahWdn u,Sdna rd Bntateffo Ms(noitcaret nniotknalpotyhp-lat ed mn,a)dnalurB( sdoht enmoitaiceps - nduaieCtapicitr aepv aed hwn,anosler ed Bneasr ohMt iswnoitaroballoc .).pe rn,pi. ltdaenalur Bt(teff od Mndanalu rhBt inwosirapmocretni e rsdouefsahc rnuopitatnemurt shn ti tiduweoir r saeacvw odbeabirc ske rdeocwnecsero u MleOfhDT d rRmaNawOr a(gsoeriPtre ploarc Pictiph Otlna et hBsegahu otodCre hdttnc ue rfjReoNh rOtnpoona s dtsn IdasesBarg a desnStanemi drneeiSt tcaiMna gdreOvlos sdieDroloC".5000179410 0:0oNN . )eIgPi d ,r.suDeBitrep olraPci tcpiOht nree BtwaoWl l tanchoaSpmI SECNEREFER t. ppn iei.rrlcpas b u a,n.drtaAnktM.aSeS f.,fWto . aM.J,nRao. k D J,l. ,e eL..u,z.PWRdoE.nKKalurB .at c.Ami h.Cla nrAof .gnit eseeMcne icciSta uO qS 9 A Ld9eoAe9htt1ttim btuc sa.r8 t 9.s 9Jbe1.AgDidruB .424 3.- m 7, i: 0 a .h8 .4. tddc5, m3J.cnaoe. i.4 AaemgJhD9t sic 9sodo1mCreouGHB e g . i.J. dr.8d reD9n.un9.aGBd14 .r6K a -.G.5rm4ae:Mh2C6 .ss e,nr.iprgona e.clO o.n8 m 9i.9Lg1n e d.h.nSZ Jae.gDidruB secn eciictS a Ou 9Lqdre9SAeoh9Atft1ti mtb cu.aserg tis db .rA,dJutn.B aaD .n,Ro ..D,GJs.rDeyB .pe r nptipircsun adm n,agniteeM .m e.h r Cra.oMp f etnrpipircsu n daGnm2a2SO: )S.1O 8(E 99.97e1gid r.u J Bdn..neDWahC . m .te prrphneoaiCirfMrpcs u: 0.dn),3Rna4t3.a m 4aJS(nO5oE7D .. 1d. 7n 4.5a 9 l -l.9 :a.7 um 1,,d4nW4r i. oan8A.5B,hAata2K .C.Lc,RKAt.aJnoD ,tanoD .R.J dna .W.C yrneH .III .7991 tcartsbA COEG 561 rof eht312 htyteico Slacimeh Cnacirem A .me h.Cr arM opfe r nptipircsun adm nganiteeM .lon m ri.oLp f etnrpipircsu n daGnm2a1SO:)1 ( S9.O78E 9.9e1gid r.u J Bd..n DGar.eKndraG Oceanogr. .lo nt prmpneoiiirfLrpcs u8dn-naCam 1:5)S 1O.S( 8O9.9E7e9g1i d .r,dJutn.B aaD .n,,Roe..DcDJirP .rg odnnaaecO , l,a.b Aa ..r,RSkt.SaJ ndo nD. ae.gJi.dDr uB .7991 .lo n. ,m6:.i9)r L95g-(o22n94a9ecO ,nai t.cmAihcom s.omCihc odoeetGttim btupsircsu n.aeMgid r.u JB d.,nDtaa n.o RD,..J A,.lSabarkS .weiver . n ,a.a m G dds...nnt1WAuan9.Su9S H1 .r.a 3M,6 .1:m-6e73h3C1 SNOITACILBUP nniobr accinag rdoevloss ifndooitubirts itdhgi erwalucel o.M89 9.1rendr a.GG .d Kn.aJ .eDgidruB .46-54 :.2m6 e.h rC.asMretawe rtonpemi deensiram eniraut s neniegort icninag rdoevloss i fdgonilc ylcacimehcoego ieb h.T89 9.1gne h .ZdS n.aJ .eDgidruB .sse r np,i.rgonae c.Olonm i.Lstnemides ytinif flaat edmezilibom m finooitaul a. v7E9 9.1nodr o.GS .dA n,aogn a.KA .,R.R .,JtanoD mo rsfdnag iglnixelpmoc-repp ogcnor tfysorevoc ed rnnaoitalo sr io)fCAM Iy(hpargotamorhc ..s 0r .,:1 er.7-eta m51naMeiwhrCam , o,g.n Aa ..K,RRt.aJ ndonD a..nSo.dAr od Gevo rnpo m iIy trdaenlvao os fci-goernreoprptosc .yhpargotamorh cytiniff alate mdezilibomm ignis usreta wenira mmor fsdnagi lgnixelpmoc .noisiv en,ri.me h.Cr aodMtettimb utspircsunaM eniraut smeo rsfdnag iglnixelpmoc-repp ofscoexu l.F79 9.1egidr u.BJ .d Dn,atan o.DR .,J.A .,SlabarkS .699- 2:9)95 (,2.4rgona e.c lO.osn tmnieLmides re pdpeov clso nsfosoiitdubir tr se.itedag w i ,ed.dt rrJna., ou.anR.,PBDo.AlDJ.aSbarkS and copper- ,t c.Amihcoms o.Cmihco e oGdtettimb utspircsu n. asMtnemid eesniraut s nesidnag iglnixelpmoc .weive rni